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期刊论文 44

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Algal biomass derived biochar anode for efficient extracellular electron uptake from

Yan-Shan Wang, Dao-Bo Li, Feng Zhang, Zhong-Hua Tong, Han-Qing Yu

《环境科学与工程前沿(英文)》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1072-5

摘要:

Algal biochar anode produced higher biocurrent compared with graphite plate anode.

Algal biochar exhibited stronger electrochemical response to redox mediators.

Algal biochar showed excellent adsorption to redox mediators.

关键词: Algal biochar     Anode material     Electrochemical activity     Extracellular electron transport     Waste resource utilization    

Mixed culture of

Kishore Gopalakrishnan, Javad Roostaei, Yongli Zhang

《环境科学与工程前沿(英文)》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1075-2

摘要:

RSM is used to explore the impact of different parameter on algal growth response.

Mixed algal culture promotes algal biomass and lipid accumulation.

Optimized conditions achieve maximum productivity of algal biomass and lipid.

关键词: Algal biofuels     Algal mixed cultures     Algal biomass     Algal lipid     Wastewater     Response surface methodology    

Cattle manure biochar and earthworm interactively affected CO and NO emissions in agricultural and forest

《环境科学与工程前沿(英文)》 2022年 第16卷 第3期 doi: 10.1007/s11783-021-1473-8

摘要:

• Earthworms increase CO2 and N2O emissions in agricultural and forest soil.

关键词: Carbon sequestration     Forest soil     Cattle manure biochar     Greenhouse gas emissions     Soil fauna    

Enhancing the adsorption function of biochar by mechanochemical graphitization for organic pollutant

《环境科学与工程前沿(英文)》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1418-2

摘要:

• Mechanochemical treatment reduced the calcination temperature for biochar synthesis.

关键词: Biochar     Mechanochemical treatment     Graphitization     Calcination temperature     Organic pollutant    

Sorption of phenanthrene to biochar modified by base

Zhengjun Feng, Lizhong Zhu

《环境科学与工程前沿(英文)》 2018年 第12卷 第2期 doi: 10.1007/s11783-017-0978-7

摘要: Biochar (BC) is a potential material for removal of polycyclic aromatic hydrocarbons from soil and water, and base modification is a promising method for improving its sorption ability. In this study, we synthesized a series of base-modified biochars, and evaluated their sorption of phenanthrene. Original biochars were produced by pyrolysis of three feedstocks (rice straw, wood and bamboo) at five temperatures (300°C, 350°C, 400°C, 500°C and 700°C). Base-modified biochars were further obtained by washing of biochars with base solution. The base soluble carbon (SC) was extracted from the supernatant, which were only obtained from biochars pyrolyzed at low temperatures (<500°C) and the content was decreased with the increase of pyrolysis temperature. The SC content between different feedstocks followed the trend of rice straw>wood>bamboo when same pyrolysis conditions were applied. It was found that base modification improved the sorption of phenanthrene on biochars that SC could be extracted from (extractable-BCs). However, base treatment but had limited effects for biochars that no SC could be extracted from. It suggested that base modification improved the sorption of phenanthrene to extractable-BCs by removing the SC and thus increasing the surface area and hydrophobicity. Therefore, base modification was suggested to be used in modifying extractable-BCs.

关键词: Biochar     Base modification     Phenanthrene    

Effects of different types of biochar on the properties and reactivity of nano zero-valent iron in soil

《环境科学与工程前沿(英文)》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1388-4

摘要:

• Biochar enhanced the mobility and stability of zero-valent iron nanoparticles.

关键词: Nano zero-valent iron     Biochar     BDE209     Transport     Soil    

Non-thermal plasma enhances performances of biochar in wastewater treatment and energy storage applications

《化学科学与工程前沿(英文)》 2022年 第16卷 第4期   页码 475-483 doi: 10.1007/s11705-021-2070-x

摘要: Surface functionalization or modification to introduce more oxygen-containing functional groups to biochar is an effective strategy for tuning the physicochemical properties and promoting follow-up applications. In this study, non-thermal plasma was applied for biochar surface carving before being used in contaminant removal and energy storage applications. The results showed that even a low dose of plasma exposure could introduce a high number density of oxygen-functional groups and enhance the hydrophilicity and metal affinity of the pristine biochar. The plasma-treated biochar enabled a faster metal-adsorption rate and a 40% higher maximum adsorption capacity of heavy metal ion Pb2+. Moreover, to add more functionality to biochar surface, biochar with and without plasma pre-treatment was activated by KOH at a temperature of 800 °C. Using the same amount of KOH, the plasma treatment resulted in an activated carbon product with the larger BET surface area and pore volume. The performance of the treated activated carbon as a supercapacitor electrode was also substantially improved by>30%. This study may provide guidelines for enhancing the surface functionality and application performances of biochar using non-thermal-based techniques.

关键词: non-thermal plasma     surface functionalization     biochar modification     wastewater treatment     supercapacitor    

Selective preparation for biofuels and high value chemicals based on biochar catalysts

《能源前沿(英文)》 2023年 第17卷 第5期   页码 635-653 doi: 10.1007/s11708-023-0878-4

摘要: The reuse of biomass wastes is crucial toward today’s energy and environmental crisis, among which, biomass-based biochar as catalysts for biofuel and high value chemical production is one of the most clean and economical solutions. In this paper, the recent advances in biofuels and high chemicals for selective production based on biochar catalysts from different biomass wastes are critically summarized. The topics mainly include the modification of biochar catalysts, the preparation of energy products, and the mechanisms of other high-value products. Suitable biochar catalysts can enhance the yield of biofuels and higher-value chemicals. Especially, the feedstock and reaction conditions of biochar catalyst, which affect the efficiency of energy products, have been the focus of recent attentions. Mechanism studies based on biochar catalysts will be helpful to the controlled products. Therefore, the design and advancement of the biochar catalyst based on mechanism research will be beneficial to increase biofuels and the conversion efficiency of chemicals into biomass. The advanced design of biochar catalysts and optimization of operational conditions based on the biomass properties are vital for the selective production of high-value chemicals and biofuels. This paper identifies the latest preparation for energy products and other high-value chemicals based on biochar catalysts progresses and offers insights into improving the yield of high selectivity for products as well as the high recyclability and low toxicity to the environment in future applications.

关键词: biomass     biochar catalysts     biofuels     high chemicals    

Adsorption of herring sperm DNA onto pine sawdust biochar: Thermodynamics and site energy distribution

《环境科学与工程前沿(英文)》 2022年 第16卷 第11期 doi: 10.1007/s11783-022-1579-7

摘要:

● Adsorption of environmental deoxyribonucleic acid on biochar was studied.

关键词: Environmental deoxyribonucleic acid     Antibiotic resistance genes     Biochar     Adsorption thermodynamics    

Erratum to: Synthesis of vinasse-dolomite nanocomposite biochar via a novel developed functionalization

《环境科学与工程前沿(英文)》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1387-5

A “Seawater-in-Sludge” approach for capacitive biochar production via the alkaline and alkaline earth

Xiling Li, Tianwei Hao, Yuxin Tang, Guanghao Chen

《环境科学与工程前沿(英文)》 2021年 第15卷 第1期 doi: 10.1007/s11783-020-1295-0

摘要: Abstract • Capacitive biochar was produced from sewage sludge. • Seawater was proved to be an alternative activation agent. • Minerals vaporization increased the surface area of biochar. • Molten salts acted as natural templates for the development of porous structure. Sewage sludge is a potential precursor for biochar production, but its effective utilization involves costly activation steps. To modify biochar properties while ensuring cost-effectiveness, we examined the feasibility of using seawater as an agent to activate biochar produced from sewage sludge. In our proof-of-concept study, seawater was proven to be an effective activation agent for biochar production, achieving a surface area of 480.3 m2/g with hierarchical porosity distribution. Benefited from our design, the catalytic effect of seawater increased not only the surface area but also the graphitization degree of biochar when comparing the pyrolysis of sewage sludge without seawater. This leads to seawater activated biochar electrodes with lower resistance, higher capacitance of 113.9 F/g comparing with control groups without seawater. Leveraging the global increase in the salinity of groundwater, especially in coastal areas, these findings provide an opportunity for recovering a valuable carbon resource from sludge.

关键词: Sewage sludge     Biochar     Seawater     Recourse recovery     Capacitor    

SPATIOTEMPORAL VARIATION OF WATER QUALITY AND ALGAL BIOMASS IN ERHAI LAKE AND ITS ENVIRONMENTAL MANAGEMENT

《农业科学与工程前沿(英文)》 2023年 第10卷 第4期   页码 566-578 doi: 10.15302/J-FASE-2023520

摘要:

Elucidating the spatiotemporal pattern of water quality and algal biomass is crucial for accurately tracing pollution sources and reducing the risk of algal blooms in lake systems. This study analyzed the spatiotemporal variability of water quality and algal biomass in Erhai Lake from 1994 to 2021 using water quality index (WQI), Mann-Kendall test and Sen’s slope combined methods. The potential causes of water quality deterioration and algal biomass dynamics were also elucidated. The results showed that the historical changes in the water environment of Erhai Lake mainly had three stages: satisfactory (1994‒2001), deteriorating (2002‒2010) and improving (2011‒2021). The changes in water quality and algal biomass were primarily affected by total nitrogen, total phosphorus and chemical oxygen demand in different stages. The water environment of Erhai Lake is currently improving significantly, starting in the southern area that is furthest from the sources of agricultural pollution, especially in summer and autumn. This is attributed to the implementation of control measures resulting in lower pollutant loads at particular times and places. Therefore, it is necessary to continue to promote standardized livestock farming, to strengthen rural wastewater collection and to investigate measures such as the interruption of the endogenous cycle.

关键词: Erhai Lake     control measures     water environment     water quality index (WQI)    

Facile fabrication of dolomite-doped biochar/bentonite for effective removal of phosphate from complex

《环境科学与工程前沿(英文)》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1671-7

摘要:

● Dolomite-doped biochar/bentonite was synthesized for phosphate removal.

关键词: Biochar-bentonite composite     Dolomite doping     Phosphate adsorption     Polymeric matrix membrane     Adsorption-filtration dual functions     Low-concentration phosphate    

Removing nitrogen and phosphorus from simulated wastewater using algal biofilm technique

WEI Qun, HU Zhiquan, LI Genbao, XIAO Bo, SUN Hao, TAO Meiping

《环境科学与工程前沿(英文)》 2008年 第2卷 第4期   页码 446-451 doi: 10.1007/s11783-008-0064-2

摘要: Algal biofilm technology is a new and advanced wastewater treatment method. Experimental study on removing nitrogen and phosphorus from simulated wastewater using algal biofilm under the continuous light of 3500 Lux in the batch and continuous systems was carried out in this paper to assess the performance of algal biofilm in removing nutrients. The results showed that the effect of removing nitrogen and phosphorus by algal biofilm was remarkable in the batch system. The removal efficiencies of total phosphorus (TP), total nitrogen (TN), ammonia-nitrogen (NH-N), and chemical oxygen demand (COD) reached 98.17%, 86.58%, 91.88%, and 97.11%, respectively. In the continuous system, hydraulic retention time (HRT) of 4 days was adopted; the effects of removing TP, TN, NH-N, and COD by algal biofilm were very stable. During a run of 24 days, the removal efficiencies of TP, TN, NH-N, and COD reached 95.38%, 83.93%, 82.38%, and 92.31%, respectively. This study demonstrates the feasibility of removing nitrogen and phosphorus from simulated wastewater using algal biofilm.

Immobilization of NZVI in polydopamine surface-modified biochar for adsorption and degradation of tetracycline

Xiangyu Wang, Weitao Lian, Xin Sun, Jun Ma, Ping Ning

《环境科学与工程前沿(英文)》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1066-3

摘要:

Novel method for polydopamine (PDA) modified biochar (BC) with immobilized NZVI.

PDA/NZVI@BC exhibits significantly enhanced activity for tetracycline (TC) removal.

TC removal efficiency was increased by 55.9% compared with that of pristine NZVI.

The mechanism of tetracycline removal by PDA/NZVI@BC was proposed.

关键词: Biochar     Polydopamine     NZVI     Modification     Tetracycline    

标题 作者 时间 类型 操作

Algal biomass derived biochar anode for efficient extracellular electron uptake from

Yan-Shan Wang, Dao-Bo Li, Feng Zhang, Zhong-Hua Tong, Han-Qing Yu

期刊论文

Mixed culture of

Kishore Gopalakrishnan, Javad Roostaei, Yongli Zhang

期刊论文

Cattle manure biochar and earthworm interactively affected CO and NO emissions in agricultural and forest

期刊论文

Enhancing the adsorption function of biochar by mechanochemical graphitization for organic pollutant

期刊论文

Sorption of phenanthrene to biochar modified by base

Zhengjun Feng, Lizhong Zhu

期刊论文

Effects of different types of biochar on the properties and reactivity of nano zero-valent iron in soil

期刊论文

Non-thermal plasma enhances performances of biochar in wastewater treatment and energy storage applications

期刊论文

Selective preparation for biofuels and high value chemicals based on biochar catalysts

期刊论文

Adsorption of herring sperm DNA onto pine sawdust biochar: Thermodynamics and site energy distribution

期刊论文

Erratum to: Synthesis of vinasse-dolomite nanocomposite biochar via a novel developed functionalization

期刊论文

A “Seawater-in-Sludge” approach for capacitive biochar production via the alkaline and alkaline earth

Xiling Li, Tianwei Hao, Yuxin Tang, Guanghao Chen

期刊论文

SPATIOTEMPORAL VARIATION OF WATER QUALITY AND ALGAL BIOMASS IN ERHAI LAKE AND ITS ENVIRONMENTAL MANAGEMENT

期刊论文

Facile fabrication of dolomite-doped biochar/bentonite for effective removal of phosphate from complex

期刊论文

Removing nitrogen and phosphorus from simulated wastewater using algal biofilm technique

WEI Qun, HU Zhiquan, LI Genbao, XIAO Bo, SUN Hao, TAO Meiping

期刊论文

Immobilization of NZVI in polydopamine surface-modified biochar for adsorption and degradation of tetracycline

Xiangyu Wang, Weitao Lian, Xin Sun, Jun Ma, Ping Ning

期刊论文